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Vasileiou or Vas[s]iliou ({{lang-gr|Βασιλείου}}) is a Greek surname. Notable people with the surname include: - Alexandros Vasileiou (1760–1818), Greek merchant and scholar
- Panagiotis Vasiliou (born 1961), Greek champion in Squash .
- Alexander Vasiliou (born 1990), Swedish-Greek artist and singer
- Alexia Vassiliou (born 1964), Cypriot singer and musician
- Androulla Vasiliou (born 1943), Cypriot and European politician
- George Vasiliou (born 1931), third President of the Republic of Cyprus
- Giorgos Vasiliou (born 1984), Cypriot footballer
- Giorgos Vasiliou (1950–2016), Greek actor
- Eleni Vasileiou (born 1974), Greek basketball player
- Maria Vassiliou (1950–1989), Cypriot actress
- Marius Vassiliou (born 1957), American geophysicist
- Michael Vasileiou, Greek merchant
- Nikos Vasiliou (born 1977), Greek footballer
- Mari Vasileiou (born 1990), Cypriot beauty pageant winner
- Spyros Vassiliou (1902–1985), Greek painter
- Stylianos Vasileiou (born 1991), Greek footballer
{{surname|Vasileiou}} 2 : Greek-language surnames|Patronymic surnames |