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词条 Neutron magnetic imaging
释义

  1. Polarized small-angle neutron scattering (SANS)

  2. Polarized neutron reflectometry

  3. Polarized Neutron Radiography and Tomography

      Precession techniques    Bulk systems    Thin film structures    Phase imaging    Scanning magnetic neutron imaging  

  4. See also

  5. References

{{Orphan|date=May 2016}}

Neutrons are spin 1/2 particles that interact with magnetic induction fields via the Zeeman interaction. This interaction is both rather large and simple to describe. Several neutron scattering techniques have been developed to use thermal neutrons to characterize magnetic micro and nanostructures.

Polarized small-angle neutron scattering (SANS)

Small-angle neutron scattering is a technique which is especially suited for the study of nanoparticles. It has for example been used extensively for the study of ferrofluids. More recently, polarized SANS has become more widely available and a wide range of study have been performed.[1][2][3] Polarized SANS allows either to probe the internal structure of magnetic nanoparticles via the measurement of the magnetic form factor or the magnetic interactions between magnetic nanoparticles via the structure factor.[4] In a few cases, Polarized Grazing Incidence SANS was performed on magnetic systems [5][6]

A few polarized neutrons SANS spectrometers are available across the world:

  • D33 at the Institut Laue-Langevin (ILL) in Grenoble France
  • PA20 at CEA Laboratoire Léon Brillouin ([https://web.archive.org/web/20090508120935/http://www-llb.cea.fr/index_e.html LLB]) in Saclay, France
  • SANS-I and KWS-1 and KWS-2 at the Forschungsneutronenquelle Heinz Maier-Leibnitz (FRM II) in Garching, Germany
  • [https://www.helmholtz-berlin.de/pubbin/igama_output?modus=einzel&sprache=en&gid=1706&typoid=39942 V4] at Helmholtz Zentrum Berlin

Polarized neutron reflectometry

Polarized neutron reflectometry allows probing magnetic thin films and ultra-thin films. The polarized reflectivity measurements allow measuring the magnitude and directions of the magnetic induction in magnetic heterostructures with a depth resolution on the order of 2-3 nm for films with thicknesses ranging from 5 to 100 nm.[7]

A number of polarized neutrons reflectometers are available across the world:

  • [https://web.archive.org/web/20080720184048/http://www.ansto.gov.au/bragg/facilities/instruments/platypus.html Platypus] at ANSTO in Sydney, Australia
  • [https://web.archive.org/web/20090218013054/http://neutron.nrc-cnrc.gc.ca/c5gen_e.html C5 spectrometer] at NRC Canada Chalk River Labs in Chalk River, Canada.
  • [https://web.archive.org/web/20090218013058/http://neutron.nrc-cnrc.gc.ca/d3gen_e.html D3 reflectometer] at NRC Canada Chalk River Labs in Chalk River, Canada.
  • D17, SuperADAM at the Institut Laue-Langevin (ILL) in Grenoble, France
  • PRISM (alternate) at CEA Laboratoire Léon Brillouin ([https://web.archive.org/web/20090508120935/http://www-llb.cea.fr/index_e.html LLB]) in Saclay, France
  • [https://web.archive.org/web/20110724150716/http://www.frm2.tum.de/wissenschaft/diffraktometer/n-rex/index.html N-REX+], [https://archive.is/20071027043123/http://www.frm2.tum.de/wissenschaft/diffraktometer/mira/index.html MIRA], [https://web.archive.org/web/20070709060558/http://www.frm2.tum.de/wissenschaft/index.html TREFF@NoSpec] and [https://web.archive.org/web/20120220025609/http://www.jcns.info/jcns_maria/ MARIA] at the Forschungsneutronenquelle Heinz Maier-Leibnitz (FRM II) in Garching, Germany
  • REFLEX and [https://web.archive.org/web/20160303210504/http://flnp.jinr.ru/139/ REMUR] at Joint Institute for Nuclear Research IBR-2 in Dubna, Russia
  • AMOR at the Paul Scherrer Institute (PSI) in Villigen, Switzerland
  • [https://web.archive.org/web/20090217073904/http://www.isis.rl.ac.uk/largescale/SURF/surf.htm SURF], CRISP{{dead link|date=June 2016|bot=medic}}{{cbignore|bot=medic}}, [https://web.archive.org/web/20090307180708/http://ts-2.isis.rl.ac.uk/instruments/inter/ INTER], [https://web.archive.org/web/20090307180724/http://ts-2.isis.rl.ac.uk/instruments/offspec/ Offspec] and [https://web.archive.org/web/20090307180729/http://ts-2.isis.rl.ac.uk/instruments/polref/ polREF] at the ISIS neutron source ([https://web.archive.org/web/20100312084955/http://www.isis.rl.ac.uk/ ISIS]) in Oxfordshire, United Kingdom
  • NG1, NG7 at the NIST Center for Neutron Research (NCNR) in Gaithersburg, Maryland, United States
  • [https://neutrons.ornl.gov/mr Magnetism] at the Spallation Neutron Source (ORNL) in Oak Ridge, Tennessee, United States

A catalogue of neutron reflectometers is available at www.reflectometry.net.

Polarized Neutron Radiography and Tomography

Precession techniques

The neutron precession in an induction field is expressed as where is the neutron magnetic moment, is the local magnetic induction at the neutron position and is the neutron gyromagnetic ratio. For neutrons, the gyromagnetic ratio is (note that for neutrons g factor is negative and equal to -3.83).

Bulk systems

Neutron radiography can be used to map the distribution of an induction field in space.[8] In order to perform such experiments, the neutron beam is initially polarized, it interacts with the induction field of interest and the neutron precession is measured with a neutron analyzer in front of the 2D detector. The beam can be either polaarized with supermirrors[9] or with polarized 3He gaz[10]

Thin film structures

The neutron precession in an induction field is rather small. Thus in the case of thin films (~1 µm thick) the neutron interaction is rather small. Thus in order to obtain a measurable signal, it has been proposed that a grazing incidence geometry could be used. In such a geometry, the interaction is enhance since the neutron travels a longer path inside the induction field. Such measurements however assume that the planar structure of the systemis homogeneous and that the induction varie only through the depth of the magnetic film. The magnetisation depth profile was measured in thick CoZr films in which the magnetic anisotropy field was "engineered" during deposition.[11] A very thorough description of the measurement process can be found in.[12]

Phase imaging

Phase contrast (or dark field) imaging has recently been developed for neutron radiography and tomography. It has been applied to vizualize magnetic domains in several types of systems:

  • soft magnetic alloys [13]
  • magnetic vortices in low Tc superconductors [14][15] superconductors [16]

Scanning magnetic neutron imaging

Magnetic neutron radiography is currently limited in spatial resolution due to the need of analyzing the neutron polarization which results in losses in spatial resolution. It has been proposed that neutron scanning imaging could be performed by using micro beams.[17][18] It is however only possible to produce 1 dimensional microbeams dur to the intrinsics limitation in neutron flux. Hence this technique can presently be applied only for 1 dimensional problems.

See also

  • Tomography
  • Tomographic reconstruction
  • Neutron Tomography

References

1. ^{{Cite journal|url = |title = Ordered arrays of magnetic nanowires investigated by polarized small-angle neutron scattering|last = Maurer|first = Thomas|date = 2014|journal = Physical Review B|volume = 89|issue = 18|pages = 184423|doi = 10.1103/physrevb.89.184423 |arxiv = 1407.7193|bibcode = 2014PhRvB..89r4423M}}
2. ^{{Cite journal|url = |title = Magnetic microstructure of a textured Nd-Fe-B sintered magnet characterized by small-angle neutron scattering|last = Perigo|first = E.A.|date = 2016|journal = Journal of Alloys and Compounds|doi = 10.1016/j.jallcom.2015.11.167|pmid = |access-date = |volume = 661|pages = 110–114}}
3. ^{{Cite journal|url = |title = Origin of Surface Canting within Fe3O4 Nanoparticles|last = Krycka|first = K.L.|date = 2014|journal = Phys. Rev. Lett.|doi = 10.1103/physrevlett.113.147203|pmid = 25325655|access-date = |volume = 113|issue = 14|pages = 147203|bibcode = 2014PhRvL.113n7203K}}
4. ^{{Cite journal|url = |title = Magnetic small-angle neutron scattering of bulk ferromagnets|last = Michels|first = A.|date = 2014|journal = Journal of Physics: Condensed Matter|doi = 10.1088/0953-8984/26/38/383201|pmid = 25180625|access-date = |volume = 26|issue = 38|page = 383201}}
5. ^{{Cite journal|url = |title = Towards a 3D magnetometry by neutron reflectometry|last = Fermon|first = C;|date = 1999|journal = Physica B: Condensed Matter|doi =10.1016/S0921-4526(99)00014-9 |pmid = |access-date = |volume = 267|issue = 1–4|pages = 162–167|bibcode = 1999PhyB..267..162F}}
6. ^{{Cite journal|url = |title = Surface diffraction on magnetic nanostructures in thin films using grazing incidence SANS|last = Pannetier|first = M.|date = 2003|journal = Physica B: Condensed Matter|doi = 10.1016/s0921-4526(03)00190-x|pmid = |access-date = |volume = 335|issue = 1–4|pages = 54–58|bibcode = 2003PhyB..335...54P}}
7. ^{{Cite journal|url = |title = Neutron reflectivity of spintronic materials|last = Zabel|first = H|date = 2006|journal = Materials Today|doi = 10.1016/S1369-7021(05)71337-7|pmid = |access-date = |volume = 9|issue = 1–2|pages = 42–49}}
8. ^{{Cite journal|url = |title = Radiography and tomography with polarized neutrons|last = Treimer|first = Wolfgang|journal = Journal of Magnetism and Magnetic Materials|doi = 10.1016/j.jmmm.2013.09.032|pmid = |access-date = |year = 2014|volume = 350|pages = 188–198|bibcode = 2014JMMM..350..188T}}
9. ^{{Cite web|url = http://www.swissneutronics.ch/fileadmin/user_upload/Dokumente/PDF/Product_Flyers/Flyer_ESS_-_polarising_devices_-_V3.pdf|title = Swiss Neutronics|date = |access-date = |website = |publisher = |last = |first = }}
10. ^{{Cite journal|url = |title = Polarized neutronimagingusinghelium-3cellsandapolychromaticbeam|last = Dawson|first = M.|journal = NIM A|doi = |pmid = |access-date = |issue = 654|year = 2011|pages = 144}}
11. ^{{Cite journal|url = |title = Probing magnetic domain wall profiles by neutron spin precession|last = Thibaudeau|first = Pascal|journal = Europhysics Letters|doi = 10.1209/0295-5075/93/37003|pmid = |access-date = |year = 2011|volume = 93|issue = 3|pages = 37003|bibcode = 2011EL.....9337003T}}
12. ^{{Cite journal|url = |title = Single domain wall chirality studies using polarised neutrons|last = Rekveldt|first = T.|date = 2013|journal = Journal of Magnetism and Magnetic Materials|doi = 10.1016/j.jmmm.2012.10.001|pmid = |access-date = |volume = 329|pages = 105–117|bibcode = 2013JMMM..329..105R}}
13. ^{{Cite journal|url = |title = Observation of Magnetic Domains in Insulation-Coated Electrical Steels by Neutron Dark-Field Imaging|last = Lee|first = Seung Wook|date = 2010|journal = Applied Physics Express|doi = 10.1143/apex.3.106602|pmid = |access-date = |volume = 3|issue = 10|page = 106602|bibcode = 2010APExp...3j6602L}}
14. ^{{Cite journal|url = |title = Three-dimensional imaging of magnetic fields with polarized neutrons|last = Kardjilov|first = N.|date = 2008|journal = Nature Physics|doi = 10.1038/nphys912|pmid = |access-date = |volume = 4|issue = 5|pages = 399–403|bibcode = 2008NatPh...4..399K}}
15. ^{{Cite journal|url = |title = Polarized neutron imaging and three-dimensional calculation of magnetic flux trapping in bulk of superconductors|last = Treimer|first = W.|date = 2012|journal = Physical Review B|doi = 10.1103/PhysRevB.85.184522|pmid = |access-date = |volume = 85|issue = 18|pages = 184522|bibcode = 2012PhRvB..85r4522T}}
16. ^{{Cite journal|title = Visualizing the morphology of vortex lattice domains in a bulk type-II superconductor|last = Reimann|first = T.|date = 2015|journal = Nature Communications|doi = 10.1038/ncomms9813|pmid = 26522610|volume = 6|page = 8813 |pmc=4667613|bibcode = 2015NatCo...6E8813R}}
17. ^{{cite journal|last1 = Ott|first1 = Frédéric|title = Shaping micron-sized cold neutron beams|journal = NIM A|date = 2015|volume = 788|pages = 29–34|doi=10.1016/j.nima.2015.03.057|bibcode = 2015NIMPA.788...29O}}
18. ^{{Cite journal|url = |title = System of neutron microbeams from a planar waveguide.|last = Kozhevnikov|first = S.K.|date = 2015|journal = JETP Letters|doi = 10.1134/s0021364015130068|pmid = |access-date = |volume = 102|issue = 1|pages = 1–6|bibcode = 2015JETPL.102....1K}}

3 : Small-angle scattering|Neutron scattering|Imaging

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